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While both enjoyed emotionally torturing their former lovers and the people in their lives making them the reigning King and Queen of Evil Exs. Katherine manipulated and killed strategically, mainly relying on useful alliances she'd charmed or seduced into doing her bidding. Katherine actions were bad but no bad enough, not by a long shot. Angelus was ultimate evil. He tortured his victims' body and soul. Drusilla is a perfect example. This quote from Buffy S2 Ep 7 (Angel telling Buffy about siring Drusilla) "First I made her insane. I killed everybody she loved, visited every mental torture on her I could devise. She eventually fled to a convent, and on the day she took her Holy Orders, I turned her into a demon."